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List of Abbreviations
Influence of CopperSulfur Covalency and CopperCopper
2Fe-2S model 3p transition analysis bonding interactions bridging sulfide calculated Chem chloride Co(II comparison contributions copper protein CsFeS2 Cu-Cu Cu-S Cu(II d-manifold d-orbital delocalization determined difference dimer dipole-allowed edge feature edge region effective nuclear charge electronic structure equation experimental Fe-S Fe(II ferredoxin ferric ferrous Hedman higher energy histidine Hodgson hydrogen bonding Inorg ionization iron atoms iron-sulfur K-edge data K-edge pre-edge K-edge spectra K-edge X-ray absorption K-edge XAS spectra ligand-metal bonding metal centers metal tetrathiolates metal-ligand metalloproteins mixed-valence model complexes molecular orbital monomer Ni(II observed oxidized Phys plastocyanin pre-edge energies pre-edge feature pre-edge intensity pre-edge peak pre-edge region pre-edge transition pseudo-Voigt redox reduction potentials renormalized Rieske protein rising edge rubredoxin scans second derivative shown in Figure solid samples Solomon spectrum Stanford Synchrotron Radiation sulfide and thiolate sulfide covalency sulfur Synchrotron Radiation Synchrotron Radiation Laboratory tetramer thiolate covalency total covalency valence versus X-ray absorption spectroscopy