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absorption ampliﬁer Appl atoms Bell Telephone Laboratories broadening California cavity cell chemical laser coefﬁcient coherent collisions crystal decay density diode discharge Doppler Doppler broadening dye laser effects efﬁciency electric electron beam emission energy equations excited experimental experiments ﬁeld ﬁrst ﬂuorescence frequency function gain glass infrared intensity interaction ionization isotope Laboratory laser beam laser operation laser output laser pulse laser pump lasing lasing threshold Lett light linear linewidth Livermore measured mirror mixture mode mode-locked modulation molecular molecules nonlinear nonlinear optical nsec observed obtained oscillator parameters peak phase photon Phys picosecond plasma polarization population inversion pressure propagation psec radiation Raman Raman Laser reﬂecting refractive refractive index resonance rotational saturable absorber saturation scattering signal spectral spectroscopy spectrum TEA laser technique temperature thermal threshold tion Torr transition tunable tuning vapor vibrational wave waveguide wavelength width x-ray