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acid Adirondack Mountains adsorbed adsorption aluminum Bh/Bhs horizons Bhs horizons Bouma calculated chemical equilibrium CO2 and DOC compartment complexity components constant degree of computation described DOC production Dokuchaev dynamics environmental equilibrium factors flux gibbsite Hoosbeek and Bryant hydraulic hypotheses i-level Models inorganic input ion exchange kaolinite kinetics layers leaching ligand losses and accumulations McBride Measured and simulated microbial decomposition mineral dissolution moisture north and south Oa horizon organic carbon parameters parent material pedodynamic model pedogenesis pedogenetic model pedology precipitation profile Figure proto-imogolite qualitative quantitative models relatively Research Richard's equation samples Simulation Model soil forming processes soil genesis soil processes soil profile Soil Sci Soil Science soil solution soil survey soil system soil temperature solid phase solute movement solute transport solution chemistry solution ratios spatial variability speciation Spodosols Sposito tensiometers thermodynamics throughfall Typic Haplorthod volumetric water content Wageningen water retention curves weathering front