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2-methylhexane 2-methylpentane 3,3-dimethylpentane azeo azeotrope boundaries azeotrope line Bancroft point binary mixtures calculated Carbon Tetrafluoride Chapter constant pressure critical endpoints critical line critical solution temperatures curve of component Davenport density double azeotrope equilibrium experimental P-T phase fluorocarbon gas-liquid critical line gas-liquid critical point gas-liquid critical temperatures Gibbs free energy given by Eq given in Fig Helmholtz free energy high pressures high-temperature hydrocarbon II-A III-l immiscibility intersection L-L to G-L LCEP LCST LCST's limited miscibility liquid phases liquid-liquid UCST low-temperature lower metastable methane miscibility mixture tube molar volume mole fraction n-heptane negative azeotropy phase behavior phase diagrams Class phase line plotted positive azeotropy Pr-Tr phase diagram pure components quadruple point Region III-HA Schematic experimental P-T shown in Fig solid boundary solubility parameter stopcock T-x diagrams temperature and pressure thermodynamic thermopile three-phase line Tr-x Tr~x phase UCEP UCEP G-L UCST's values vapor pressure curve volume Waals equation