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activated complex Acuchem adsorbed adsorption group adsorption of Rj aldehyde algebraic Analytical solutions Arrhenius pre-exponential factor associative adsorption autoxidation bimolecular bimolecular reaction Boudart Chem Chemical Kinetics Chemisorption collision frequency concentrations consider constant-volume batch reactor database Delplot rank Delplot Technique desorption developed differential equations Eley-Rideal energy equilibrium example expression for ROO first-rank Delplot Heterogeneous Catalysis Heterogeneous Catalytic Reactions higher rank products illustrate Intercept invoke the QSSA KpPp L/mol-s line of centers linear simple MARI molecules network rank overall reaction P+ K P+ phase primary products product rank Pyrolysis quasi-equilibrium Rank Delplots rate coefficients rate constant expression rate determining step rate expression rate law reacting system reaction controlling reaction coordinate reaction mechanism reaction network Reaction Pathway reaction rate law reactions involving reactive intermediate reverse reactions SbH3 second-rank Delplot simple collision theory surface thermochemical thermodynamics transition state theory two-step write rate laws zero