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absorption coefficient activation energy amidogen ammonia ammonia decomposition approximately assumed band Beer's Law boron trichloride calculated carbon dioxide cell Chem chemical reactions collision partners constant convection corresponds density detection deuterium diameter dl/dx energy transfer equation equilibrium et.al excited experiments Figure frequency function gases heat capacity heat conduction heat transfer heated ammonia heated region hydrogen incident power increase infrared input window iridium isotope effect kcal kcal/mole kinetic laser beam laser heated laser illumination laser induced chemistry laser irradiation laser radiation light emission light intensity Losev measured meters micron mixture mode molecular observed optical oscilloscope photon Phys plot pressure broadened processes production pulse pumped reaction rate reduced mass schlieren shock tube species spectrometer spontaneous emission temperature dependence temperature distribution theory thermal conductivity torr transition translational temperature tungsten tungsten filament vibrational energy vibrational relaxation watts watts/cm yield