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amplitude factor anisotropic axis bilayer biphasic region Blinc C-D bond calculated CDCl Chem components contribution correlation function Cryst cutoff frequency DEB-d2 in 8CB DEB-dg densities of motion density matrix determined deuterium deuterons DF model diffusion equation EFG tensor elastic constants Euler angles EXCESS experimental exponential extreme narrowing FORTRAN Freed frequency dependence G.R. Luckhurst G.W. Gray Hamiltonian hydrodynamic inversion-recovery isotropic phase kcal kcal mol"1 Larmor frequency lattice layer liquid crystals listed in Table measured MINPACK molecular reorientation molecular symmetry motional models nematic phase nonselective observed order parameter corrections ordered phases partially ordered phase transition Phya Phys probe molecule quadrupolar quadrupolar interaction R.R. Void R.Y. Dong Relaxation Data relaxation studies reorientational motion restoring potential rotational diffusion equation shown in Fig slow motions smectic phases solute molecules spectral densities spherical spin-lattice relaxation SRLS model static order parameter symmetry T1IR temperature dependence values viscosity coefficient