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Axial Nitroxide in an Axial PotentialModel
Fluctuating Torques 509
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analysis anisotropic viscosity asymmetric potential axes axis system basis set BEPC BOCP Brownian diffusion C/B ratio calculated components contribution correlation function coupled coefficients defined by Eq dependent diagonal diffusion equation discussed effects eigenfunctions eigenvalues Euler angles evaluated experimental Figure fluctuating torques frequency gauss given by Eq Hamiltonian hyperfine included isotropic liquids isotropic phase jump diffusion lineshapes linewidth Liouville equation liquid crystals magnetic parameters magnetic tensors Maier-Saupe potential Markov operator matrix elements MBBA mesophase molecular orientation molecule motional narrowing region nematic phase nitroxide non-secular terms Note observed obtained odd L values ordering parameter PDT in Phase perturbation theory principal axis principal axis system proton pseudosecular terms quantum number relaxation reorientation residual linewidth rigid limit Section II.F.2.d shown simulated slow motional slow tumbling solvent spectra spectral densities spectrum spin Hamiltonian stochastic Liouville strong jump Table TCNE temperature tion tonian transitions z-axis