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Electron transfer mediated by glucose oxidase at the liquidliquid interface
Biomaterial engineered electrodes for bioelectronics
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acid active adsorbed adsorption Anal aqueous Au-electrode azurin biosensors catalytic current catalytic response cathodic cell chains charge Chem chemical Chemistry complex concentration copper proteins covalent cyclic voltammetry cyclic voltammograms cytochrome b5 detection diffusion domains electroactive electrochemical electrochemistry electrode surface electron transfer electrostatic enzyme experimental experiments F. A. Armstrong FADH2 Faraday Discuss ferrocene glucose oxidase gold electrode H. A. O. Hill haem heme heme edge heme propionate hydrogen peroxide hydrophobic immobilised interactions interface interfacial electron transfer kinetics layer ligands lipid measured mediator membrane modulation Moiroux mol cm"2 molecular molecules monolayer mutant NarGH nitrate observed obtained oxygen peak peroxidase phosphate buffer polylysine polymer potential step potentiostat present Prof proton QH-ADH rate constant reaction redox potential reduction potential scan rate Scheme sensor shown in Fig shows solution species structure studies substrate surfactant wild type Willner