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Thermal versus optical transitions
Methods for studying electronic structure at very high
Electronic transitions in metals and insulatormetal
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100 PRESSURE 3d orbitals 50 kbar acceptor acetylacetonate anthracene approximation aromatic atomic back donation backbonding behavior bonding Bridgman charge transfer peak Chem chemical complexes compounds conduction band configuration interaction conversion covalency crystal field decrease diketones discussed in Chapter donor electrical resistance electronic transitions Equation excited exhibit Fe(II FePc ferric ion ferrous ion function of pressure H. G. DRICKAMER half width hematin hemin high pressure product high spin hydrocarbons imidazole increasing pressure intermediate spin involves iron isomer shift kbar kbar Fig lattice ligand field ligand field theory low pressure low spin lower energy MCWHAN measurements metal ion molecular orbital molecules Mossbauer resonance Mossbauer spectra observed octahedral optical absorption overlap oxidation parameters pentacene perylene phenanthroline phthalocyanine Phys porphyrin protons quadrupole splitting reduction relative rings shown in Fig Solids spectrum spin ferrous structure symmetry temperature theory thermal occupation transition metal valence band wave functions