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absolute density adsorption bulb American chemical society angstrom units apparatus area and pore-size Area of Graphite artificial graphite atomic products operation burette calculated Clausius-Clapeyron equation crystalline expansion decrease upon irradiation density of artificial density of graphite desorption isotherms determined differential heat Effects of Radiation electric company electron volts empty pore space entropy experimental extrusion axis Figure gas adsorbed gases given graphite sample given sample graphite crystallites graphite decreases Hanford atomic products heat of adsorption helium gas displacement irradiated graphite irradiated samples layer liquid nitrogen low temperature irradiation manometer mz/gm nitrogen gas Outgassing Temperature oxygen physical Pile graphite pore-size distribution curves porous Powder pulverized quartz quartz containers radiation flux Relative Pressure Richland samples exposed shrinkage studies surface area surface area increased surface characteristics surface covered Table Temperature Area transition barrier type of graphite types of artificial V-Vm virgin and irradiated VIRGIN SAMPLE WSF WSF WSF x-ray diffraction