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absorption ampliﬁer amplitude anti-Stokes Appl atoms band broadening cavity cell Chem CO2 laser coherent collisions color center crystal decay density dependence detection distribution dye laser effects efﬁciency electron emission energy equation excimer laser excitation exciton experimental experiments ﬁeld ﬁrst ﬂuence ﬂuorescence four-wave mixing interaction ionization irradiation Laboratory laser beam laser frequency laser intensity laser pulse laser pumped Lett linear linewidth measured medium mode modulation molecular molecules multiphoton nonlinear nonlinear optical observed obtained optical bistability optical pumping oscillator output parameters peak phase conjugate photon Phys picosecond plasma polarization probe quantum reﬂectivity refractive index resonance rotational sample saturated absorption saturation semiconductor shown in Fig shows signal spatial spectra spectroscopy spectrum stimulated emission streak camera surface target technique temperature thermal threshold transition tunable tuned two-photon USA PACS velocity vibrational wave waveguide wavelength width