## Band shapes and correlation functions from infrared and Raman spectra of some symmetric top liquids |

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### Contents

Theory | 7 |

Experimental Methods and Analysis | 30 |

Band Shapes and Correlation Functions | 41 |

6 other sections not shown

### Common terms and phrases

angular momentum average jump angle band of CD^I band shapes bands studied benzene benzyl alcohol Boltzmann distribution boundary conditions CD3I CH^CN CH^I and CD^I CH3CN CH3I cJJJ(t classical values correlated error CROT(t dependence depolarized Rayleigh determined dielectric constant Doctor of Philosophy Figure free rotation step free rotor frequency functions for band functions for v3 given molecule infrared and Raman infrared rotational infrared spectroscopy measured molecular motion molecular reorientation molecular symmetry molecule rotates obtain perpendicular polarizability polarized psec pure liquids Raman and infrared Raman scattering ratio Rayleigh scattering relation functions rH rH ROT-IR rotational correlation function rotational diffusion model rotational jump model rotational relaxation second moments Shapes and Correlation short time behavior solution spectrometer Stokes symmetric top molecule symmetry axis SYSTEM BAND temperature theory v3 band values of M(2 vibrational correlation functions viscometer viscosity width