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absorption spectrum anharmonic atoms bacteriorhodopsin band beam broadening cavity dye laser cell Chem coherent configuration crystal decay density density matrix dependence dephasing detection detector dielectric relaxation dissociation DMST dye laser effects electronic emission energy transfer equation excitation spectrum experimental experiments field fluorescence ground harmonic infrared inhomogeneous intensity interaction intramolecular ionization ions isotope laser excitation laser pulse Lett lifetime lines linewidth manifold measured method mode mode-locked molecular molecules multiphoton nonradiative observed obtained one-photon optical oscillator pentacene perturbations phase photochemistry photodissociation photoluminescence photon Phys picosecond picosecond pulses polarization polarization spectroscopy pressure probe psec pump quantum yield Rabi frequency radiative coupling Raman spectroscopy Range relaxation resolution rotational saturated absorption saturation short cavity dye shown in Figure signal single singlet solution solvent spectra studies technique temperature tetrazine time-resolved tion transition triplet tunable tuned two-photon vibrational wavelength width Zewail