Studies in Energy Transfer: I. Vibrational Relaxation of Carbon Dioxide by Water and Heavy Water; II. Carbon Dioxide Laser Irradiation of Ammonia |
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absorption coefficient activation energy amidogen ammonia ammonia decomposition approximately assumed Beer's Law boron trichloride calculated cell Chem chemical reactions CO₂ CO2 laser CO₂-H₂O collision partners constant convection corresponds D₂ D₂O density detection deuterium diameter energy transfer equation equilibrium excited experiments Figure frequency gases H₂ H₂O heat capacity heat conduction heat transfer heated ammonia heated region incident power increase infrared input window iridium isotope effect kcal kcal/mole kinetic laser beam laser heated laser induced chemistry laser induced light laser irradiation laser radiation light emission light intensity measured meters micron mixture molecular msec N₂ NH₂ observed oscilloscope photon Phys plot pressure broadened processes production pulse pumped reaction rate reduced mass S. H. Bauer schlieren shock tube temperature dependence temperature distribution theory thermal conductivity torr transition translational temperature tungsten tungsten filament vibrational energy vibrational relaxation watts watts/cm