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acetic acetonitrile acid addition alkyl amines analysis Angew anion Anklam aqueous aromatic atom barrier benzene calculations carbanions carbenium ions carbocations carbon carbonyl catalysis catalyzed Chem chemical shifts chirality chloride complex compounds concentration conformations conjugate correlation cyclic cycloaddition Department of Chemistry dependence derivatives determined discussed dissociation electron transfer energy enthalpy equilibrium esters ether experimental formation gas phase hydrogen bonding hydrolysis initio Institute interaction intermediates intramolecular investigated ion pairs isomer isomerization Japan kcal/mol ketones KINETIC ISOTOPE EFFECTS ligand measured mechanism mechanistic methanol method methyl mixture MNDO moiety molecular molecules nitrogen nucleophilic observed obtained Organic Chemistry Organische Chemie oxidation oxygen parameters phenyl photochemical polar proton proton transfer rate constants ratio reaction reactivity rearrangement resonance ring rotation salts solution solvation solvent solvolysis species spectra spectroscopy stabilization stereochemistry steric studied substituent effects substituents substrate synthesized temperature thermodynamic triplet Universitat University values vinyl cations