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absorption adjusted alignment amplifier axis background FWM CARS cell combination band contribution correlation function coupling cross-peaks crystal delay stage density matrix dephasing detection detector DOVE-IR DOVE-Raman electric field electronic equation excitation experiments factor Figure fluctuations focused frequency domain frequency scanned fundamental FWM intensity gate Gaussian geometry heterodyning homodyne detection homogeneous broadening important infrared inhomogeneous input pulses interactions interference involving laser linewidth method mirror modes molecular monochromator natural narrowing non-linear spectroscopy optical optical Bloch equations oscillator output frequency parameters paths peak perturbation phase-matching photon photon echo picosecond pinhole polarization population processes pump pure dephasing quantum beating Rabi frequency Raman Raman spectroscopy ratio refraction regenerative amplifier resonant response function result retroreflector rime sample setup simulations solution solvent spectra spectrum Spitfire techniques temporal discrimination transition dipoles TRIVE TRTVE ultrafast up-conversion vibrational spectroscopy wavevector width zero