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absorption amount applied aqueous attached average broad calculated cations CHAPTER Chem comparing complex compressibility concentration constant containing Coord coordinated methanol coordination number cps separation crystals decrease density described determining solvation numbers dielectric effective entropy environments equilibrium quotient exchange expected experimental factor Figure forming frequency hydration hydration number hydroxyl proton hydroxyl proton absorp included Increasing Magnetic Field interpretation ionic ions isotopic dilution kinds known lower magnesium measurements method mole of salt moles CH moles of methanol moles of water moles water NMR Proton Spectrum nuclear magnetic resonance observed peaks perchlorate Phys possible primary solvation number probably range reference relative represented respectively result samples shell shifted shows side Sol'n solution solvation sphere solvent molecules Stanford University structure studied TABLE taken Taube temperature term tion transfer transport ultrasonic viscosity volume water content water molecules water per mole X-ray